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GROMACS+PLUMED pre-2023 vs. 2024+ give very different exchange proabilities with PT-WTE #1384

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@rcrehuet

We have found a troubling beaviour when running PT-WTE simulations: despite using identical system configurations, force fields, and biasing parameters, the exchange probabilities between replicas differ dramatically between the two GROMACS versions:
Exchange Probabilities (Biasing Phase)

  • GROMACS 2023:

    Average exchange probability: 0.070 ± 0.010
    Range: 0.05 - 0.09
    All 30 inter-replica exchanges show consistently low acceptance rates

  • GROMACS 2024.3:

    Average exchange probability: 0.314 ± 0.044
    Range: 0.22 - 0.38
    All 30 inter-replica exchanges show consistently high acceptance rates

Overall increase: ~4.5x increase in average exchange probability when using GROMACS 2024.3

This plot shows the exchange probabilities between 31 replicas:

Image

The energy distributions are also different between the two gromacs versions, but surprisingly gromacs 2023 produces larger fluctuations than 2024:

Image

All the files needed to reproduce the simulations are available in this Zenodo repository: https://doi.org/10.5281/zenodo.19203432.
The outputs of the 2023 and 2024 versions are also there, together with a jupyter notebook with more analysis and plots.

We believe that this issue is related to this one.

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